According to the Intel web site, the Intel Matrix Storage Manager does NOT support array expansion.
Even if it did, it would be highly unlikely that you would be able to expand your partition beyond 2TB unless you had originally formatted the partition as GPT type. To be more specific, you may be able to get the array beyond 2TB but you would need to create additional partitions to use the additional capacity.
Velocity Micro Cinemagix Grand Theater, C2Q, 2GB, 2 TB, 3 DCT, 2 HDHomeRun
Homebuilt C2Q, 2 GB, 1.5 TB, HVR-1600, FireSTB
Dell E1705, T7600, 2GB, 250GB, HVR-950
WHS, WRT600N, DMA-2100, DMA-2200, XBox360